| Don Messick | Papa Smurf | |
| Lucille Bliss | Smurfette | |
| Michael Bell | Handy Smurf | |
| Hamilton Camp | Greedy Smurf | |
| Paul Winchell | Gargamel | |
| Alan Young | Farmer Smurf |
| Danny Goldman | Brainy Smurf | |
| Frank Welker | Hefty Smurf | |
| June Foray | Jokey Smurf | |
| William Callaway | Clumsy Smurf | |
| Alan Oppenheimer | Vanity Smurf | |
| Kip King | Tailor Smurf |